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Oxygen-induced doping on reduced PEDOT

Overview of attention for article published in Journal of Materials Chemistry, January 2017
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  • In the top 25% of all research outputs scored by Altmetric
  • Good Attention Score compared to outputs of the same age (77th percentile)
  • High Attention Score compared to outputs of the same age and source (92nd percentile)

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2 X users
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2 patents

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106 Mendeley
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Title
Oxygen-induced doping on reduced PEDOT
Published in
Journal of Materials Chemistry, January 2017
DOI 10.1039/c6ta10521a
Pubmed ID
Authors

E. Mitraka, M. J. Jafari, M. Vagin, X. Liu, M. Fahlman, T. Ederth, M. Berggren, M. P. Jonsson, X. Crispin

Abstract

The conducting polymer poly(3,4-ethylenedioxythiophene) (PEDOT) has shown promise as air electrode in renewable energy technologies like metal-air batteries and fuel cells. PEDOT is based on atomic elements of high abundance and is synthesized at low temperature from solution. The mechanism of oxygen reduction reaction (ORR) over chemically polymerized PEDOT:Cl still remains controversial with eventual role of transition metal impurities. However, regardless of the mechanistic route, we here demonstrate yet another key active role of PEDOT in the ORR mechanism. Our study demonstrates the decoupling of conductivity (intrinsic property) from electrocatalysis (as an extrinsic phenomenon) yielding the evidence of doping of the polymer by oxygen during ORR. Hence, the PEDOT electrode is electrochemically reduced (undoped) in the voltage range of ORR regime, but O2 keeps it conducting; ensuring PEDOT to act as an electrode for the ORR. The interaction of oxygen with the polymer electrode is investigated with a battery of spectroscopic techniques.

X Demographics

X Demographics

The data shown below were collected from the profiles of 2 X users who shared this research output. Click here to find out more about how the information was compiled.
Mendeley readers

Mendeley readers

The data shown below were compiled from readership statistics for 106 Mendeley readers of this research output. Click here to see the associated Mendeley record.

Geographical breakdown

Country Count As %
Unknown 106 100%

Demographic breakdown

Readers by professional status Count As %
Student > Ph. D. Student 22 21%
Researcher 16 15%
Student > Master 11 10%
Student > Bachelor 9 8%
Student > Doctoral Student 7 7%
Other 10 9%
Unknown 31 29%
Readers by discipline Count As %
Chemistry 31 29%
Materials Science 16 15%
Engineering 8 8%
Physics and Astronomy 6 6%
Chemical Engineering 5 5%
Other 10 9%
Unknown 30 28%
Attention Score in Context

Attention Score in Context

This research output has an Altmetric Attention Score of 7. This is our high-level measure of the quality and quantity of online attention that it has received. This Attention Score, as well as the ranking and number of research outputs shown below, was calculated when the research output was last mentioned on 28 May 2020.
All research outputs
#5,271,264
of 25,756,911 outputs
Outputs from Journal of Materials Chemistry
#1,754
of 19,298 outputs
Outputs of similar age
#96,187
of 424,022 outputs
Outputs of similar age from Journal of Materials Chemistry
#88
of 1,202 outputs
Altmetric has tracked 25,756,911 research outputs across all sources so far. Compared to these this one has done well and is in the 79th percentile: it's in the top 25% of all research outputs ever tracked by Altmetric.
So far Altmetric has tracked 19,298 research outputs from this source. They receive a mean Attention Score of 3.1. This one has done particularly well, scoring higher than 90% of its peers.
Older research outputs will score higher simply because they've had more time to accumulate mentions. To account for age we can compare this Altmetric Attention Score to the 424,022 tracked outputs that were published within six weeks on either side of this one in any source. This one has done well, scoring higher than 77% of its contemporaries.
We're also able to compare this research output to 1,202 others from the same source and published within six weeks on either side of this one. This one has done particularly well, scoring higher than 92% of its contemporaries.