Title |
A hole-conductor–free, fully printable mesoscopic perovskite solar cell with high stability
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Published in |
Science, July 2014
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DOI | 10.1126/science.1254763 |
Pubmed ID | |
Authors |
Anyi Mei, Xiong Li, Linfeng Liu, Zhiliang Ku, Tongfa Liu, Yaoguang Rong, Mi Xu, Min Hu, Jiangzhao Chen, Ying Yang, Michael Grätzel, Hongwei Han |
Abstract |
We fabricated a perovskite solar cell that uses a double layer of mesoporous TiO2 and ZrO2 as a scaffold infiltrated with perovskite and does not require a hole-conducting layer. The perovskite was produced by drop-casting a solution of PbI2, methylammonium (MA) iodide, and 5-ammoniumvaleric acid (5-AVA) iodide through a porous carbon film. The 5-AVA templating created mixed-cation perovskite (5-AVA)x(MA)1- xPbI3 crystals with lower defect concentration and better pore filling as well as more complete contact with the TiO2 scaffold, resulting in a longer exciton lifetime and a higher quantum yield for photoinduced charge separation as compared to MAPbI3. The cell achieved a certified power conversion efficiency of 12.8% and was stable for >1000 hours in ambient air under full sunlight. |
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United States | 6 | 33% |
United Kingdom | 2 | 11% |
Thailand | 1 | 6% |
Australia | 1 | 6% |
Norway | 1 | 6% |
India | 1 | 6% |
Unknown | 6 | 33% |
Demographic breakdown
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Scientists | 1 | 6% |
Mendeley readers
Geographical breakdown
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United Kingdom | 9 | <1% |
Belgium | 6 | <1% |
Japan | 5 | <1% |
Germany | 5 | <1% |
Korea, Republic of | 3 | <1% |
France | 2 | <1% |
Netherlands | 2 | <1% |
Australia | 2 | <1% |
Other | 20 | <1% |
Unknown | 2038 | 97% |
Demographic breakdown
Readers by professional status | Count | As % |
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Student > Ph. D. Student | 592 | 28% |
Researcher | 324 | 15% |
Student > Master | 283 | 13% |
Student > Bachelor | 151 | 7% |
Student > Doctoral Student | 103 | 5% |
Other | 297 | 14% |
Unknown | 360 | 17% |
Readers by discipline | Count | As % |
---|---|---|
Materials Science | 481 | 23% |
Chemistry | 384 | 18% |
Physics and Astronomy | 299 | 14% |
Engineering | 260 | 12% |
Energy | 115 | 5% |
Other | 113 | 5% |
Unknown | 458 | 22% |