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3D electrogenerated chemiluminescence: from surface-confined reactions to bulk emission

Overview of attention for article published in Chemical Science, January 2015
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Title
3D electrogenerated chemiluminescence: from surface-confined reactions to bulk emission
Published in
Chemical Science, January 2015
DOI 10.1039/c5sc01530h
Pubmed ID
Authors

Milica Sentic, Stéphane Arbault, Laurent Bouffier, Dragan Manojlovic, Alexander Kuhn, Neso Sojic

Abstract

Among luminescence techniques, electrogenerated chemiluminescence (ECL) provides a unique level of manipulation of the luminescent process by controlling the electrochemical trigger. Despite its attractiveness, ECL is by essence a 2D process where light emission is strictly confined to the electrode surface. To overcome this intrinsic limitation, we added a new spatial dimension to the ECL process by generating 3D ECL at the level of millions of micro-emitters dispersed in solution. Each single object is addressed remotely by bipolar electrochemistry and they generate collectively the luminescence in the bulk. Therefore, the entire volume of the solution produces light. To illustrate the generality of this concept, we extended it to a suspension of multi-walled carbon nanotubes where each one acts as an individual ECL nano-emitter. This approach enables a change of paradigm by switching from a surface-limited process to 3D electrogenerated light emission.

X Demographics

X Demographics

The data shown below were collected from the profiles of 2 X users who shared this research output. Click here to find out more about how the information was compiled.
Mendeley readers

Mendeley readers

The data shown below were compiled from readership statistics for 47 Mendeley readers of this research output. Click here to see the associated Mendeley record.

Geographical breakdown

Country Count As %
Spain 1 2%
Netherlands 1 2%
France 1 2%
Unknown 44 94%

Demographic breakdown

Readers by professional status Count As %
Student > Ph. D. Student 10 21%
Researcher 7 15%
Student > Doctoral Student 3 6%
Professor > Associate Professor 3 6%
Student > Master 3 6%
Other 7 15%
Unknown 14 30%
Readers by discipline Count As %
Chemistry 13 28%
Engineering 4 9%
Unspecified 2 4%
Environmental Science 1 2%
Biochemistry, Genetics and Molecular Biology 1 2%
Other 4 9%
Unknown 22 47%
Attention Score in Context

Attention Score in Context

This research output has an Altmetric Attention Score of 2. This is our high-level measure of the quality and quantity of online attention that it has received. This Attention Score, as well as the ranking and number of research outputs shown below, was calculated when the research output was last mentioned on 21 July 2015.
All research outputs
#13,747,855
of 22,817,213 outputs
Outputs from Chemical Science
#5,283
of 7,813 outputs
Outputs of similar age
#178,118
of 353,112 outputs
Outputs of similar age from Chemical Science
#360
of 492 outputs
Altmetric has tracked 22,817,213 research outputs across all sources so far. This one is in the 38th percentile – i.e., 38% of other outputs scored the same or lower than it.
So far Altmetric has tracked 7,813 research outputs from this source. They typically receive more attention than average, with a mean Attention Score of 7.6. This one is in the 31st percentile – i.e., 31% of its peers scored the same or lower than it.
Older research outputs will score higher simply because they've had more time to accumulate mentions. To account for age we can compare this Altmetric Attention Score to the 353,112 tracked outputs that were published within six weeks on either side of this one in any source. This one is in the 48th percentile – i.e., 48% of its contemporaries scored the same or lower than it.
We're also able to compare this research output to 492 others from the same source and published within six weeks on either side of this one. This one is in the 26th percentile – i.e., 26% of its contemporaries scored the same or lower than it.