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Electrocatalytic Oxygen Evolution with an Immobilized TAML Activator

Overview of attention for article published in Journal of the American Chemical Society, April 2014
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About this Attention Score

  • In the top 25% of all research outputs scored by Altmetric
  • High Attention Score compared to outputs of the same age (80th percentile)
  • Good Attention Score compared to outputs of the same age and source (70th percentile)

Mentioned by

blogs
1 blog

Citations

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54 Dimensions

Readers on

mendeley
72 Mendeley
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1 CiteULike
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Title
Electrocatalytic Oxygen Evolution with an Immobilized TAML Activator
Published in
Journal of the American Chemical Society, April 2014
DOI 10.1021/ja5015986
Pubmed ID
Authors

Ethan L. Demeter, Shayna L. Hilburg, Newell R. Washburn, Terrence J. Collins, John R. Kitchin

Abstract

Iron complexes of tetra-amido macrocyclic ligands are important members of the suite of oxidation catalysts known as TAML activators. TAML activators are known to be fast homogeneous water oxidation (WO) catalysts, producing oxygen in the presence of chemical oxidants, e.g., ceric ammonium nitrate. These homogeneous systems exhibited low turnover numbers (TONs). Here we demonstrate immobilization on glassy carbon and carbon paper in an ink composed of the prototype TAML activator, carbon black, and Nafion and the subsequent use of this composition in heterogeneous electrocatalytic WO. The immobilized TAML system is shown to readily produce O2 with much higher TONs than the homogeneous predecessors.

Mendeley readers

The data shown below were compiled from readership statistics for 72 Mendeley readers of this research output. Click here to see the associated Mendeley record.

Geographical breakdown

Country Count As %
Mexico 1 1%
United States 1 1%
Unknown 70 97%

Demographic breakdown

Readers by professional status Count As %
Student > Ph. D. Student 29 40%
Researcher 14 19%
Student > Bachelor 7 10%
Student > Master 6 8%
Student > Doctoral Student 3 4%
Other 10 14%
Unknown 3 4%
Readers by discipline Count As %
Chemistry 57 79%
Materials Science 2 3%
Chemical Engineering 2 3%
Engineering 2 3%
Computer Science 1 1%
Other 3 4%
Unknown 5 7%

Attention Score in Context

This research output has an Altmetric Attention Score of 6. This is our high-level measure of the quality and quantity of online attention that it has received. This Attention Score, as well as the ranking and number of research outputs shown below, was calculated when the research output was last mentioned on 12 August 2016.
All research outputs
#1,572,145
of 8,204,367 outputs
Outputs from Journal of the American Chemical Society
#5,087
of 19,053 outputs
Outputs of similar age
#35,413
of 178,675 outputs
Outputs of similar age from Journal of the American Chemical Society
#136
of 472 outputs
Altmetric has tracked 8,204,367 research outputs across all sources so far. Compared to these this one has done well and is in the 80th percentile: it's in the top 25% of all research outputs ever tracked by Altmetric.
So far Altmetric has tracked 19,053 research outputs from this source. They typically receive a little more attention than average, with a mean Attention Score of 5.3. This one has gotten more attention than average, scoring higher than 73% of its peers.
Older research outputs will score higher simply because they've had more time to accumulate mentions. To account for age we can compare this Altmetric Attention Score to the 178,675 tracked outputs that were published within six weeks on either side of this one in any source. This one has done well, scoring higher than 80% of its contemporaries.
We're also able to compare this research output to 472 others from the same source and published within six weeks on either side of this one. This one has gotten more attention than average, scoring higher than 70% of its contemporaries.