Title |
Photoluminescence enhancement of quantum dots on Ag nanoneedles
|
---|---|
Published in |
Discover Nano, August 2012
|
DOI | 10.1186/1556-276x-7-438 |
Pubmed ID | |
Authors |
Syed Rahin Ahmed, Hee Ryoung Cha, Jung Youn Park, Enoch Y Park, Dongyun Lee, Jaebeom Lee |
Abstract |
Noble metal nanostructure allows us to tune optical and electrical properties, which has high utility for real-world application. We studied surface plasmon-induced emission of semiconductor quantum dots (QDs) on engineered metallic nanostructures. Highly passive organic ZnS-capped CdSe QDs were spin-coated on poly-(methyl methacrylate)-covered Ag films, which brought QDs near the metallic surface. We obtained the enhanced electromagnetic field and reduced fluorescence lifetimes from CdSe/ZnS QDs due to the strong coupling of emitter wave function with the Ag plasmon resonance. Observed changes include a six-fold increase in the fluorescence intensity and striking reduction in fluorescence lifetimes of CdSe/ZnS QDs on rough Ag nanoneedle compared to the case of smooth surfaces. The advantages of using those nanocomposites are expected for high-efficiency light-emitting diodes, platform fabrication of biological and environmental monitoring, and high-contrast imaging. |
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Geographical breakdown
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Unknown | 38 | 95% |
Demographic breakdown
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Researcher | 5 | 13% |
Student > Postgraduate | 4 | 10% |
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Professor | 4 | 10% |
Other | 8 | 20% |
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Other | 0 | 0% |
Unknown | 12 | 30% |